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Volume 1
Contains:
- "The Legion of Super-Heroes" Adventure 247,
April 1958
- "Prisoner of the Super-Heroes" Adventure
267, December 1959
- "The Three Super-Heroes" Action 267, August
1960
- "The Army of Living Kryptonite Men" Superboy
86, January 1961
- "Lana Lang and the Legion of Super-Heroes" Adventure
282, March 1961
- "Supergirl's Three Super-Girl Friends" Action
276, May 1961
- "Superboy's Big Brother" Superboy 89, June
1961
- "The Legion of Super-Villains" Superman
147, August 1961
- "The Secret of the Seventh Super-Hero" Adventure
290, November 1961
- "The Legion of Super-Traitors" Adventure
293, February 1962
- "Supergirl's Greatest Challenge" Action
287, April 1962
- "Superman's Super-Courtship" Action 289,
June 1962
- "The Boy with Ultra-Powers" Superboy 98,
July 1962
- "The Face Behind the Lead Mask" Adventure
300, September 1962
- "The Secret Origin of Bouncing Boy" Adventure
301, October 1962
- "Sun Boy's Lost Poswer" Adventure 302, November
1962
- "The Fantastic Spy" Adventure 303, December
1962
- "The Stolen Super-Powers" Adventure 304,
January 1963
- "The Secret of the Mystery Legionnaire" Adventure
305, February 1963
(not available)
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Volume 2
Contains:
- "The Legion of Substitute Heroes" Adventure
306, March 1963
- "The Secret Power of the Mystery Super-Hero" Adventure
307, April 1963
- "The Return of Lightning Lad" Adventure
308, May 1963
- "The Legion of Super Monsters" Adventure
309, June 1963
- "The Doom of the Super-Heroes" Adventure
310, July 1963
- "The War Between the Substitute Heroes and the Legion"
Adventure 311, August 1963
- "The Super-Sacrifice of the Legionnaires" Adventure
312, September 1963
- "The World of Doomed Olsens" Jimmy Olsen
72, October 1963
- "The Condemned Legionnaires" Adventure 313,
October 1963
- "The Super-Villains of All Ages" Adventure
314, November 1963
- "The Legionnaires' Super-Contest" Adventure
315, December 1963
- "The Renegade Super-Hero" Adventure 316,
January 1964
- "The Menace of Dream Girl" Adventure 317,
February 1964
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Volume 3
Contains:
- "The Mutiny fo the Legionnaires" Adventure
318, March 1964
- "Elastic Lad Jimmy and His Legion Romances" Jimmy
Olsen 76, April 1964
- "The Legion's Suicide Squad" Adventure 319,
April 1964
- "The Revenge of the Knave From Krypton" Adventure
320, May 1964
- "The Code of the Legion" Adventure 321,
June 1964
- "The Super-Tests of the Super-Pets" Adventure
322, July 1964
- "The Eight Impossible Missions" Adventure
323, August 1964
- "The Legion of Super-Outlaws" Adventure
324, September 1964
- "Lex Luthor Meets the Legion of Super-Heroes" Adventure
325, October 1964
- "Revolt of the Girl Legionnaires" Adventure
326, November 1964
- "Superboy and the Five Legion Traitors" Superboy
117, December 1964
- "The Lone Wolf Legionnaire" Adventure 327,
December 1964
- "The Lad Who Wrecked the Legion" Adventure
328, January 1965
(not available)
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Volume 4
Contains:
- "The Bizarro Legion" Adventure 329, February
1965
- "Secret of the Mystery Legionnaire: Adventure
330, March 1965
- "Thre Triumph of the Legion of Super-Villains"
Adventure 331, April 1965
- "The Super-Moby Dick of Space" Adventure
332, May 1965
- "The War Between Krypton and Earth" Adventure
333, June 1965
- "The Unknown Legionnaire" Adventure 334,
July 1965
- "Starfinger" Adventure 335, August 1965
- "The True Identity of Starfinger" Adventure
336, September 1965
- "The Insect Queen of Smallville" Superboy
124, October 1965
- "The Weddings that Wrecked the Legion" Adventure
337, October 1965
- "The Meance of the Sinister Space-Babies" Adventure
338, November 1965
- "The Sacrifice of Kid Psycho" Superboy 125,
December 1965
- "Hunters of the Super-Beasts" Adventure
339, December 1965
(not available)
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Volume 5
Contains:
- "Computo the Conqueror" Adventure 340, January
1966
- "The Weirdo Legionnaire" Adventure 341,
February 1966
- "The Legionnaire Who Killed" Adventure 342,
March 1966
- "The Evil Hand of the Luck Lords" Adventure
343, April 1966
- "The Super-Stalag of Space" Adventure 344,
May 1966
- "The Execution of Matter-Eater Lad" Adventure
345, June 1966
- "One of Us is a Traitor" Adventure 346,
July 1966
- "The Traitor's Triumph" Adventure 347, August
1966
- "Target - 21 Legionnaires" Adventure 348,
September 1966
- "The Rogue Legionnaire" Adventure 349, October
1966
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Volume 6
Contains:
- "The Outcast Super-Heroes" Adventure 350,
November 1966
- "The Forgotten Legion" Adventure 351, December
1966
- "The Fatal Five" Adventure 352, January
1967
- "The Doomed Legionnaire" Adventure 353,
February 1967
- "The Adult Legion" Adventure 354, March
1967
- "The War of the Legions" Adventure 355,
April 1967
- "The Six-Legged Legionnaire" Adventure 355,
April 1967
- "The Five Legion Orphans" Adventure 356,
May 1967
- "The Ghost of Ferro Lad" Adventure 357,
June 1967
- "The Hunter" Adventure 358, July 1967
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Volume 7
Contains:
- "The Outlawed Legionnaires" Adventure 359,
August 1967
- "The Legion Chain Gang" Adventure 360, September
1967
- "The Unkillables" Adventure 361, October
1967
- "The Lone Wolf Legionnaire Reporter" Jimmy Olsen
106, October 1967
- "The Chemoids Are Coming" Adventure 362,
November 1967
- "Black Day for the Legion" Adventure 363,
December 1967
- "The Revolt of the Super-Pets" Adventure
364, January 1968
- "Escape of the Fatal Five" Adventure 365,
February 1968
- "The Fight for the Championship of the Universe"
Adventure 366, March 1968
- "No Escape From the Circle of Death" Adventure
367, April 1968
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Volume 8
Contains:
- "The Mutiny of the Super-Heroines" Adventure
368, May 1968
- "The Origin of the Legion" Superboy 147,
May-June 1968
- "Mordru the Merciless" Adventure 369, June
1968
- "The Devil's Jury" Adventure 370, July 1968
- "The Colossal Failure" Adventure 371, August
1968
- "When Superboy Walked Out on the Legion" Adventure
371, August 1968
- "School for Super-Villains" Adventure 372,
September 1968
- "The Tornado Twins" Adventure 373, October
1968
- "Mission: Diabolical" Adventure 374, November
1968
- "The King of the Legion" Adventure 375,
December 1968
- "The Execution of Chameleon Boy" Adventure
376, January 1969
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